OH1晶体中级联光学差频效应产生太赫兹波

Terahertz generation by OH1 based on cascaded difference frequency generation

  • 摘要: 理论分析了有机晶体2-3-(4-hydroxystyryl)-5,5-dimethylcyclohex-2-enylidenemalononitrile(OH1)中基于共线相位匹配级联光学差频产生太赫兹波的物理过程。从耦合波方程出发分析了级联斯托克斯过程和级联反斯托克斯过程,计算了太赫兹波的强度和量子转换效率。相对于非级联光学差频过程,13阶级联光学差频产生的太赫兹波强度增大了15.96倍。13阶级联光学差频中太赫兹波的量子转换效率为1377%,超过了Manley-Rowe关系的限制。

     

    Abstract: Terahertz(THz) wave generation by organic crystal 2-3-(4-hydroxystyryl)-5,5-dimethylcyclohex-2-enylidenemalononitrile(OH1) with a collinear phase-matching scheme based on cascaded difference frequency generation(DFG) processes was theoretically analyzed. The cascaded Stokes interaction processes and the cascaded anti-Stokes interaction processes were investigated from coupled wave equations. THz intensities and quantum conversion efficiency were calculated. Compared with non-cascaded DFG processes, THz intensities from 13-order cascaded DFG processes were increased to 15.96. The quantum conversion efficiency of 1 377% in cascaded processes can be realized, which exceeds the Manley-Rowe limit.

     

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